The effect of diamond-like carbon (DLC) coating (fabricated by cathodic arc deposition) on mechanical properties, tribological behavior and corrosion performance of the Ni−Al−bronze (NAB) alloy was investigated. Nano-hardness and pin-on-plate test showed that DLC coating had a greater hardness compared with NAB alloy. Besides, the decrease in friction coefficient from 0.2 for NAB substrate to 0.13 for the DLC-coated sample was observed. Potentiodynamic polarization and EIS results showed that the corrosion current density decreased from 2.5 µA/cm2 for bare NAB alloy to 0.14 µA/cm2 for DLC-coated sample in 3.5 wt.% NaCl solution. Moreover, the charge transfer resistance at the substrate−electrolyte interface increased from 3.3 kΩꞏcm2 for NAB alloy to 120.8 kΩꞏcm2 for DLC-coated alloy, which indicated an increase in corrosion resistance due to the DLC coating