In this paper, the spectrophotometric properties of a colored Nickel-based solution complex (Nickel nitrate hexahydrate and Methyl Orange (MO)) were investigated as a stable chemical dosimeter with a simple synthesis and low cost for use in radiation processing. The maximum absorbance for the solution was observed at 460 nm. This solution was irradiated at three different concentrations of Ni(No3)2.6H2O and MO by Co-60 gamma-ray. The results showed the solution absorbance decreases with an increase in doses, and this solution can be used as a routine dosimeter and has a linear response in the 50 to 1500 Gy range with acceptable repeatability and stability in environmental conditions up to 40 days before and after irradiation.