This investigation presents a unified theoretical framework that combines coupledcluster nuclear structure calculations with time-dependent density functional theory (TDDFT) to describe both ground-state properties and dynamical processes in atomic nuclei. The chiral effective field theory (EFT) Hamiltonian up to N3LO provides the foundation for structure calculations, whereas the time-dependent extension of the Skyrme energy density functional treats large-amplitude collective motion. For stable nuclei up to 78Ni, coupled-cluster calculations reproduce binding energies within 1% accuracy and predict charge radii that agree with recent precision measurements. In the actinide region, time-dependent simulations quantitatively reproduced fission fragment distributions and kinetic energy spectra, revealing a 15% reduction in descent time due to dynamical pairing correlations. For 240Pu fission, the calculations reproduce the experimental fragment mass distributions with 92% accuracy. The ab initio structure calculations provide ground-state densities and pairing fields that initialize the TDDFT dynamics, ensuring consistency across energy scales. This coupling is demonstrated through the reproduction of both static properties and dynamical observables. These results establish a crucial connection between microscopic nuclear structures and macroscopic collective dynamics, while identifying specific areas that require improved treatment of three-nucleon forces and continuum couplings.
